双层石墨烯的到点特性和透光特性
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Optical conductance and transmission in bilayer graphene
H. M. Dong, J. Zhang, F. M. Peeters, and W. Xu
Citation: J. Appl. Phys. 106, 043103 (2009); doi: 10.1063/1.3200959
View online: http://dx.doi.org/10.1063/1.3200959
View Table of Contents: http://jap.aip.org/resource/1/JAPIAU/v106/i4
Published by the American Institute of Physics.
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Downloaded 22 Dec 2012 to 140.124.249.101. Redistribution subject to AIP license or copyright; see http://jap.aip.org/about/rights_and_permissionsOpticalconductanceandtransmissioninbilayergraphene
H.M.Dong,1J.Zhang,2F.M.Peeters,3andW.Xu1,2,a͒1KeyLaboratoryofMaterialsPhysics,InstituteofSolidStatePhysics,ChineseAcademyofSciences,Hefei230031,China2DepartmentofPhysics,YunnanUniversity,Kunming610015,China3DepartmentofPhysics,UniversityofAntwerp,Groenenborgerlaan171,B-2020Antwerpen,Belgium
͑Received5May2009;accepted10July2009;publishedonline20August2009͒
Wepresentatheoreticalstudyoftheoptoelectronicpropertiesofbilayergraphene.Theoptical
conductanceandtransmissioncoefficientarecalculatedusingtheenergy-balanceequationderived
fromaBoltzmannequationforanair/graphene/dielectric-wafersystem.Forshortwavelengths͑Ͻ0.2m͒,weobtaintheuniversalopticalconductance=e2/͑2ប͒.Interestingly,thereexistsan
opticalabsorptionwindowinthewavelengthrange10–100m,whichisinducedbydifferent
transitionenergiesrequiredforinter-andintra-bandopticalabsorptionsinthepresenceofthe
Moss–Bursteineffect.Asaresult,thepositionandwidthofthisabsorptionwindowdepend
sensitivelyontemperature,carrierdensity,andsamplemobilityofthesystem.Theseresultsare
relevantforapplicationsofrecentlydevelopedgraphenedevicesinadvancedoptoelectronicssuch
astheinfraredphotodetectors.©2009AmericanInstituteofPhysics.͓DOI:10.1063/1.3200959͔
I.INTRODUCTION
Grapheneisthebasisofanewclassofnanostructures
whereconductionoccursinsingleorfewlayersofcarbon
atomsarrangedinahexagonallattice.1Owingtoitsunique
electronicbandstructureandthecorrespondingquasirelativ-
isticfeatures,graphenehasattractedagreatattentioninre-
centyears.Furthermore,graphenecanhaveahighcarrier
densityandexhibitshighelectronicmobilityevenatroom
temperature.Oneofthemajoradvantagesofagraphenede-
viceisthatthecarrierdensityinthegraphenelayercanbe
controlledveryeffectivelythroughagatevoltage.1Hence,
graphenehasbeenproposedasa“buildingblock”forad-
vancedelectronicdevices2suchasgraphenep-nandp-n-p
junctions,3transistors,4etc.Inrecentyears,thestudyofthe
electronictransportpropertiesofDiracquasiparticlesin
graphenehasrapidlybecomeanimportantresearchtopicin
nanomaterialscience,condensedmatterphysics,and
nanoelectronics,5whichispartlymotivatedbythepossible
applicationsofgrapheneinadvancedelectronicdevices.6
Recently,theopticalandoptoelectronicpropertiesofdif-
ferentgraphenesystemshavebeeninvestigated.Inparticu-
lar,itwasfoundexperimentallythattheopticalconductance
pergraphenelayerisgivenbyauniversalvalue
=e2/͑4ប͒inthevisiblefrequencyandUVrange.7Asacon-
sequence,thelighttransmittanceofmonolayerandbilayer
graphenedevicesareabout0.98and0.96,respectively,inthe
visiblebandwidth.8Thisimportantdiscoveryhasresultedin
theproposalthatgraphenecanbeusedtoreplaceconven-
tionalindiumtinoxideelectrodesformakingbetterand
cheaperopticaldisplays.9Kuzmenkoetal.7recentlyfound
experimentallythatforphotonenergysmallerthan0.2eV,
thereisanopticalabsorptionwindow.Thewidthanddepth
ofthiswindowdependstronglyontemperature.Thisinter-
estingfindingimpliesthatgraphenemayalsobeappliedforinfrareddetectioninambientcondition.Veryrecentexperi-
mentalworkshowedthatgraphenecanhavestrongintra-
andinter-bandtransitionswhichcanbesubstantiallymodi-
fiedthroughelectricalgating,similartoresistancetuningin
graphenefield-effecttransistors.10Theseexperimentalresults
showclearlythatgraphenecanbeusednotonlyasadvanced
electronicdevicesbutalsoasopticaldevicesforvariousap-
plications.
Inconjunctionwithexperimentalinvestigationsintoop-
toelectronicpropertiesofgraphenesystems,theoreticalstudy
inthisareahasbeenquiteactive.Theuniversalopticalcon-
ductanceinthevisibleregime,0=e2/4បpergraphenelayer,
hasbeenobtainedtheoretically.7,11Thefeaturesofgraphene
systemsunderfar-infrared͑FIR͒orterahertzradiationhave
alsobeeninvestigatedtheoreticallyusingvarious
approaches.12,13Theresultsobtainedfromthesetheoretical
investigationshaveindicatedthat͑i͒intheshortwavelength
suchasvisibleregime,inter-bandtransitionistheprincipal
channelforopticalabsorptionandconductancein
graphene;7,11͑ii͒intheFIRorterahertzbandwidth,both
inter-andintra-bandtransitionsplayimportantrolestocause
opticalabsorptionandconductanceingraphene;12,13and͑iii͒
theoptoelectronicpropertiesforgrapheneintheFIRortera-
hertzregimedependstronglyontemperatureandcarrierden-
sityinthesystem.12
Theopticalandoptoelectronicpropertiesofmonolayer
graphenehasbeenwelldocumented.7,8,10Incontrasttoa
nearlylinearenergyspectruminmonolayergraphene,bi-
layergraphenehasaquadraticenergyspectruminlowen-
ergyregime.14,15Thus,thedensityofstatesinabilayer
graphenesystemdifferssignificantlyfromthatinmonolayer
graphene.Ithasbeenrealizedthatbilayergrapheneisof
equalimportanceasmonolayergrapheneforbothtechno-
logicalapplicationsandfundamentalscience.4,16Inthispa-
perwepresentadetailedtheoreticalstudyoftheoptoelec-
tronicpropertiesofbilayergraphene.InSec.II,the
theoreticalapproachisdevelopedtocalculatetheoptoelec-a͒Electronicmail:wenxu_issp@yahoo.cn.JOURNALOFAPPLIEDPHYSICS106,043103͑2009͒
0021-8979/2009/106͑4͒/043103/6/$25.00©2009AmericanInstituteofPhysics106,043103-1
Downloaded 22 Dec 2012 to 140.124.249.101. Redistribution subject to AIP license or copyright; see http://jap.aip.org/about/rights_and_permissions